unfriend

[ uhn-frend ]

verb (used with object)

to remove (a person) from one's list of friends, or contacts, on a social media website.

Origin of unfriend

2005–10; un-² + friend (in the sense “to add to one's list of contacts”)

Unfrien′dedness, the state of being unfriended; Unfrien′dliness, unkindness; unfriend′ship, unfriendliness.
Chambers's Twentieth Century Dictionary (part 4 of 4: S-Z and supplements) | Various
But I have told thee all these things to show that the King is not without some reason to be thy father's unfriend.
Men of Iron | Howard Pyle
The Queen said that she could not be content that either he or any else should be unfriend to Moray.
The Mystery of Mary Stuart | Andrew Lang
Item, Gif it beis askit, in caise the Castell be unfriend, whair the armye shalbe placed?
The Works of John Knox, Volume 2 (of 6) | John Knox
You are dealing with an emissary from a foreign power who is an unfriend of my country.
Astounding Stories of Super-Science January 1931 | Various

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